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《Journal of Safety and Environment》 2007-02
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On the research advances in China for degradating pentachlorophenol

LI Meng-yao, LI Wei-liang , QIAN Hui(School of Environmental Science and Engineering, Chang'anUniversity, Xi'an 710054, China)  
The present paper is aimed at giving an introductory review of the recent advances in the pentachlorophenol treatment. As is known, pentachlorophenol is one of the organic pollutants (POPs) with harmful properties of being toxic, semi-volatile, bio-accumulative as well as persistent in the environment and human bodies. It is just for the above reasons and some others not mentioned here, it is of great significance to study how to better degrade the contamination and pollution it has brought and would bring to the environmental contamination. For the given research purpose, this paper has made a review over the great advances in recent years in treating pentachlorophenol in China. So far as we know, chemical and biological methods have rather widely been used in PCP degradation. However, photocatalyst and electronic irradiation methods have mainly been adopted for the chemical degradation. In addition, the paper have also made careful comparisons among several photocatalyst treating technologies, including UV, UV/H2O2, UV/H2O2/Fe(Ⅱ/Ⅲ), UV/TiO2 and the merits and demerits from the point of view of the different methods' efficiency, influencing factors, intermediates and reaction mechanism. The chemical degradation mechanism lies in the free radical oxidation and chlorine replacement with hydroxyl and PCP by transforming polyphenol or quinone, then opening the rings and finally mineralizing them. Last of all, discussion has been also extended to the screening of microbes, degradation paths and mechanism with PCP biodegradation. Under aerobic conditions, PCP starts by hydrolytic para-hydroxylation, and then yielding chlorinated para-hydroquinone. As a matter of fact, the anaerobic biodegradation of PCP occurs by reductive dechlorination, a process by which chlorine can be replaced with hydrogen and part of intermediate being finally transformed into CH4 and CO2.
【Fund】: 国家自然科学基金资助项目“水溶液平衡化学模拟及其水文地球化学应用研究”(40372114)
【CateGory Index】: X592
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