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《Journal of Jilin University(Earth Science Edition)》 2011-04
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Characteristic Comparison of Hydrocarbon Generation Kinetics Under Open-Closed Systems with Constant Heating Rates and Its Significance

LI Ting-ting1,WANG Min1,2,LU Shuang-fang1,TIAN Shan-si1,CHEN Guo-hui1,HAN Lu31.College of Earth Sciences,Northeast Petroleum University,Daqing 163318,Heilongjiang,China2.Key Laboratory of Tectonics and Petroleum Resources(China University of Key Laboratory of Geosciences),Ministry of Eduction,Hubei Province,Wuhan 430074,China3.College of Horticulture Science and Technology,Hebei Normal University of Science and Technology,Qinhuangdao 066004,Hebei,China  
In order to reveal the difference of hydrocarbon generation kinetics characteristics and its geologic application under different experiment conditions,two thermal simulation apparatus(open and closed systems) are employed to pyrolyze coal sample from Songliao basin.According to the relationship between experimental product yields and temperature,the kinetic models of the oil/gas generated from organic matter are calibrated.Then the kinetic parameters obtained from two experimental systems are extrapolated under the experimental heating rate and the geological heating rate,the results show that the TR(transformation ratio) increasing rate of the gas generation under closed system is slower than that under open system,the reason is that the coal sample pyrolysis to gas under open system is mainly primary cracking,but under closed system it is a common result of primary and secondary cracking.For further application,the hydrocarbon generation threshold is calculated,which combined the burial-thermal history of Xujiaweizi and the kinetic parameters obtained from two experimental systems.And the extrapolation result shows that the calculated geological time(115 Ma) corresponding to the threshold from open system is earlier than the geological time corresponding to the actual threshold(110 Ma),and the calculated geological time(92 Ma) corresponding to the threshold from closed system is later than the geological time corresponding to the actual threshold.
【Fund】: 国家自然科学基金项目(40972101);; 国家油气重大专项(2008ZX05007-001 2008ZX05004-003);; 国家重点基础研究发展计划项目(2009CB219306);; 教育部重点实验室开放课题(TPR-2010-23)
【CateGory Index】: P618.13
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