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《Chinese Journal of Catalysis》 2004-01
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Study on the Photocatalytic Hydrolysis of Methylacetylene under Visible Light Irradiation Ⅱ. Effect of Vanadium Ion on Performance of Titania Photocatalyst

ZHANG Jinlong 1* , CHEN Haijun 1, XU Huasheng 1, Masakazu ANPO 2(1 Institute of Fine Chemicals, East China University of Science and Technology, Shanghai 200237, China; 2 Department of Applied Chemistry, Graduate School of Engineering, Osaka Prefecture University, 1 1 Gakuen cho, Sakai, Osaka 599 8531, Japan)  
The photocatalytic performance of some kinds of titania photocatalyst with different grain size for hydrolysis of methylacetylene under visible light irradiation was investigated. The results showed that using ion implantation was able to extend photo absorption regions of nano photocatalyst, resulting in the shift of absorption band of titania photocatalyst to visible light, and the extent of shift increased with increasing titania grain size. Especially, the implantation of V ion made the photocatalyst possessing catalytic activity in the region of visible light. After implantation of V ion, the photocatalytic activity of titania catalyst did not decrease in the UV region but increase in the visible light region. Among the five kinds of photocatalyst, V ion implanted P 25 with middle grain size exhibits the highest photocatalytic activity. These kinds of photocatalyst also possessed high catalytic activity under solar light irradiation.
【Fund】: 国家自然科学基金资助项目 (2 0 0 73 0 2 6);; 教育部科技重点项目;; 上海市教委曙光计划;; 上海市纳米发展与促进中心纳米专项资助
【CateGory Index】: O643.3
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1 ZHANG Jinlong 1* , XU Huasheng 1, Masakazu ANPO 2(1 Institute of Fine Chemicals, East China University of Science and Technology, Shanghai 200237, China; 2 Department of Applied Chemistry, Graduate School of Engineering, Osaka Prefect ure University, 1-1 Gakuen-cho, Sakai, Osaka 599-8531, Japan);Study on the Photocatalytic Hydrolysis of Methylacetylene under UV Light Irradiation Ⅰ. Performance of Nano-titania Photocatalyst[J];催化学报;2003-11
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