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《Chinese Journal of Catalysis》 2006-01
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Preparation of Highly Active Cr_2O_3-SiO_2 Catalyst by Sol-Gel Method for Ethylbenzene Dehydrogenation in the Presence of CO_2

LI Huiyun 1,3, YUE Yinghong1, MIAO Changxi2, XIE Zaiku2, HUA Weiming 1*, GAO Zi1(1 Department of Chemistry and Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Fudan University, Shanghai 200433, China; 2 Shanghai Research Institute of Petrochemical Technology, SINOPEC, Shanghai 201208, China; 3 Department of Chemistry, Anyang Teachers College, Anyang 455002, Henan, China)  
The Cr_2O_3-SiO ? catalyst was prepared by a sol-gel method. It displays two times higher catalytic activity for the dehydrogenation of ethylbenzene in the presence of CO_2 than the regular SiO_2-supported chromia catalyst.The higher amount of Cr 6+ present in the former catalyst accounts for its superior catalytic performance in the dehydrogenation reaction.
【Fund】: 国家重点基础研究发展规划(2000077507);; 上海市重大基础研究(03DJ14004);; 国家自然科学基金(20303004);; 上海市自然科学基金(03ZR14013);; 上海石油化工研究院资助项目.
【CateGory Index】: O643.32
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【References】
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1 CHEN Shuwei1,2,QIN Zhangfeng1,SUN Ailing1,WANG Jianguo1, 1State Key Laboratory of Coal Conversion,Institute of Coal Chemistry,The Chinese Academy of Sciences,Taiyuan 030001,Shanxi,China;2College of Chemistry and Chemical Engineering,Taiyuan University of Technology,Taiyuan 030024,Shanxi,China;Effects of Li Promoter on the Catalytic Performance of Fe-Li/AC for Ethylbenzene Dehydrogenation in the Presence of CO_2[J];Chinese Journal of Catalysis;2009-04
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【Co-citations】
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1 ZHU Xiangxue 1, ZHANG Shibo 2, QIAN Xinhua 2, NIU Xionglei 1, SONG Yueqin 1, LIU Shenglin 1, XU Longya 1* (1 Dalian Institute of Chemical Physics, The Chinese Academy of Sciences, Dalian 116023, Liaoning, China; 2 Fushun Petrochemical Company, CNPC, Fushun 113008, Liaoning, China);Effects of Steam Treatment on Acidity of ZSM-5 and Its Catalytic Performance in Butene Cracking[J];Chinese Journal of Catalysis;2004-07
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3 TAO Weichuan~ 1,2 , MAO Dongsen~ 2* , CHEN Qingling~ 1,2 , HU Ying~1(1 Chemical and Pharmaceutical Institute, East China University of Science and Technology, Shanghai 200237, China;2 Shanghai Research Institute of Petrochemical Technology, SINOPEC, Shanghai 201208, China);Effect of Post-treatment of Silicalite-1 on Its Catalytic Performance for Vapor-Phase Beckmann Rearrangement of Cyclohexanone Oxime[J];Chinese Journal of Catalysis;2005-05
4 ZHAO Guoliang~(1,2),TENG Jiawei~2,XIE Zaiku~2,TANG Yi~(1*),YANG Weimin~2,CHEN Qingling~2(1 Department of Chemistry,Fudan University,Shanghai 200433,China;2 Shanghai Research Institute of Petrochemical Technology,SINOPEC,Shanghai 201208,China);Characterization and Catalytic Performance of(NH_4)_2SiF_6-Modified HZSM-5 Catalyst for C_4 Olefin Cracking[J];Chinese Journal of Catalysis;2005-12
5 LI Wenying*, LI Xiaohong, SONG Ruiwei(Key Laboratory of Coal Science and Technology for Ministry of Education and Shanxi Province, Taiyuan University of Technology, Taiyuan 030024, Shanxi, China);V-Doped Titanium Mixed Oxide Catalysts for Oxidative Dehydrogenation of Ethylbenzene with CO_2[J];Chinese Journal of Catalysis;2006-12
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9 YE Xingnan 1,2 , HUA Weiming 1, YUE Yinghong 1, MIAO Changxi 3, XIE Zaiku 3, GAO Zi 1* (1 Department of Chemistry and Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Fudan University, Shanghai 200433, China; 2 School of Pharmacy, Fudan University, Shanghai 200032, China; 3 Shanghai Research Institute of Petrochemical Technology, SINOPEC, Shanghai 201208, China);Ethylbenzene Dehydrogenation to Styrene in the Presence of Carbon Dioxide over Supported Chromia Catalysts[J];Chinese Journal of Catalysis;2004-07
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