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《Acta Sedimentologica Sinica》 1991-01
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Isotopic Geochemistry of Nonhydrocarbons in Natural Gas from Sanshui Basin, Guangdong

Du Jianguo Liu Wenhui Song Minliang (Lanzhou Institute of Geology. Chinese Academy of Seiences.)  
Based on geochemical characteristics of stable helium, argon, carbon and nitrogen isotopes for natural gas, origins of nonhydrocarbons and fluids are discussed. 3He/4He ratios in natural gas are 1.14-4.54 times as much as that in the air. Stable isotope compositions of argon of natural gas are rich in 40Ar (40Ar/ 36Ar=450-841) .Carbon isotope compositions (δ13CPDB) of carbon dioxide vary from-20‰ to -2‰.The δ15 Nvalues of natural gases range between -57.7‰ and 95.1‰.The values (Q) of heat fluid in the Sanshui Basin calculated depend on He "He ratios, change from 72 mWm to 82 mWm-2.The high values of heat fluid and isotopic ratios of He. Ar. C and N have a relation to ancient volcanos. The geochemical qualities of stable isotopes of He, Ar, C and N in natural gases indicate that there are strong deep (matter and heat) fluids in the Sanshui basin.Part of He, Ar and N in some reservoirs came from the mantle. Nonhydrocarbons originated from the crust are mixed in various kinds of natural gases. Carbon dioxide in natural gases is mainly originated from the crust, CO2 depleted in 13C is mainly originated from degradation of organic matter in strata; but CO2 enriched in 13C are from reaction between carbonate rocks and under ground water and thermal fluids, and mixed in CO2 from the deep earth. An amount of heat fluid was derived from the upper mantle.
【Fund】: 国家自然科学基金委资助项目 0488013
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