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《Acta Sedimentologica Sinica》 2002-03
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The Influence of High Pressure on the Structural and Compositional Evolution of Natural Bitumen

GAO Zhi-nong HU Hua-zhong (College of Chemistry and Molecular Sciences, Wuhan University, Wuhan 430072)  
Laboratory simulation has elucidated that high pressure (800~1 000 atm) at moderate temperatures (300~500 ℃) can accelerate the structural evolution of natural bitumen in carbonate rocks. Under high pressures, the natural bitumen becomes more compact and regular in its structures. So the reflectance values (R b) of bitumen increase obviously, and its R b values and structural parameters (carbon lamellar distance d 002, size of crystal nucleus, layer number of aromatic cycle and aromaticity) exceed that in the real thermal evolution level evidently. Nevertheless, this kind of bitumen preserves the chemical composition and distribution (including biomarkers) formed in true thermal maturity. This unique geochemical nature differs from that of any published bitumen types (e.g., thermally matured bitumen, etc.), which can be used to distinguish thermo-compressively matured bitumen from other kinds of bitumens.
【Fund】: 湖北省自然科学基金 (2 0 0 0J0 2 3);; 国家九五科技攻关项目 (96 1 1 1 0 3 0 4和 96 1 1 0 0 2 0 4 0 1 )资助
【CateGory Index】: P618.13
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