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《Acta Sedimentologica Sinica》 2003-01
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Evolution of Carbon Isotopic Composition in Pyrolytic Gases Generated from Coal and Its Main Macerals

LIU Wen-hui1 SONG Yan2 LIU Quan-you1 QIN Sheng-fei2 WANG Xiao-feng1 1(State Key Laboratory of Gas Geochemistry, Lanzhou Institute of Geology, Chinese Academy of Sciences, Lanzhou 730000) 2(Research Institute of Petroleum Exploration and Development, CNPC, Beijing 100083)  
Simulation experiment is an important part in the study on organic geochemistry. It is also an important means for the research of oil and gas geochemistry. According to the analysis of component and isotope composition of pyrolytic gases generated from simulation of coal and its main macerals, we replenish and perfect the predecessor's cognition of isotopic composition in pyrolytic gases generated from simulation in this paper. Moreover, we contrastively study the fractional characteristics of carbon isotope in coal-type gases and pyrolytic gases, and the result shows that they have favourable consistency. Basing on careful simulation, we can gain the decisive index of coal-type gases generated from different coal-bearing sedimentary basin. To the contrast of carbon isotopic composition between natural gases and simulation gases, what the most important is how to deal with the isotopic analysis data. According to the carbon isotope analysis of the simulation series products, we obtain the relationship between methane, ethane carbon isotopic composition and evolution stage in natural gas with single source, and the relationship between methane carbon isotope and ethane carbon isotope in evolution process. All of these results have an important significance to judgie gases of mixed sources.
【Fund】: 国家自然科学基金 (批准号 :499730 10 );; 中国科学院重点方向 ( KZCX2 -111)联合资助
【CateGory Index】: P593
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