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《GEOCHIMICA》 1999-04
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A two stage model of carbon isotopic fractionation in coal gas

Liu Wenhui Xu Yongchang(State Key Laboratory of Gas Geochemistry,Lanzhou Institute of Geology,Chinese Academy of Sciences, Lanzhou 73000)  
Carbon isotopic composition of methane in natural gas is one of the most effective indicators to identify the type of source rock and the stage of its evolution. The relationships between δ13C1 of coal gas and Ro(vitrinite reflectance) of the relevant source rocks have been studied extensively in the world and important results have been obtained. But owing to the limitation of the object of individual research, the comprehensive model of isotopic fractionation during the evolutions of gas and source rock needs to be further developed. Because of the widespread coal seam and the completeness of hydrocarbon generation and evolution of the source rocks in China, systematic study of the whole evolution is possible. In this paper, through the studies of carbon isotopic composition methane in coal gas and the evolution degree of relevant source rocks in different evolution stages and different geological age of source rocks in different basins in China, the two stage model of carbon isotopic fractionation of methane in coal gas was obtained by using the mathematical regression and the analysis of a lot of other information. The mechanism of this fractionation was probed as well. This model will play an important role in exploring and developing coal gases, especially those generated at lower evolutionary stages.
【Fund】: 中国科学院兰州地质研究所气体地球化学国家重点实验室资助
【CateGory Index】: P597
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