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《Geochimica》 2001-06
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A study of activation energy of coal macerals

SUN Xu guang1, QIN Sheng fei2, LUO Jian2, JIN Kui li3(1. Department of Geology, Peking University, Beijing 100871, China; 2. Beijing Institute of Petroleum Exploration and Development, Beijing 100083, China;3.Beijing Graduate School, China University o  
The parameters of kinetic (such as activation energy) of maceral isonly related to the chemical structure of maceral itself. Therefore, like fingerprint, the parameters of kinetic of maceral can indicate the chemical structureof different macerals. Rock Eval and Py GC are used to study the relationship between activation energy and hydrocarbon generation rate of barkinite, vitrinite and fusinite. The results show that the activation energy distributions of barkinite, vitrinite and fusinite are very different. For barkinite, 77%of the pyrolysis products correspond to the activation energy of 162.5~175 kJ/mol. However, vitrinite and fusinite show a distinctive bimodal or multimodal distribution model, 64%and 24%of the pyrolysis products from vitrinite correspondto the activation energy of 191.25 ~198 kJ/mol and more than 211.25 kJ/mol. For fusinite, 49%and 15%of pyrolysis products correspond to the activation energy of 250~262.5 kJ/mol and more than 662.5 kJ/mol, respectively. These indicate that the chemical structure of barkinite, desmocollinite and fusinite are very different. Generally, the narrower the hydrocarbon generation activation energy range, the more uniform of the maceral organic composition is. Adversely, the wider the range of hydrocarbon generation activation energy, the more complexorganic composition would be. Based on these, it can be concluded that the chemical composition of barkinite is simpler than that of vitrinite and fusinite. The chemical structures of barkinite are mainly composed of aliphatic compounds, and contain a few aromatic structures. However, vitrinite are mostly composed of methyloxydibenzene, and fusinite are mainly composed of ethyloxybenzene and ethylbenzene, propylbenzene, besides these, there also contain a few short chain alkane and heterocyclic compound. In addition, the average activation energy of the three macerals is very different, so the "oil window"of barkinite, vitrinite and fusinite are different. The average activation energy of barkinite, vitrinite and fusinite are 177 kJ/mol, 200 kJ/mol and 360 kJ/mol, respectively, based on these, it can be concluded that hydrocarbon generating sequence of the three macerals are barkinite, vitrinite, fusinite.
【Fund】: 国家自然科学基金(49672131;40102014)
【CateGory Index】: P632
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