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《Geochimica》 2006-04
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Effect of montmorillonites from different localities on photocatalytic activity of surfactants modified TiO_2 pillared montmorillonites

AN Tai-cheng1,YUAN Jian-mei2,CHEN Jia-xin1,ZENG Xiang-ying1,CHEN Hui 2,SHENG Guo-ying1,FU Jia-mo1 and YU Xiao-lan3 1.State Key Laboratory of Organic Geochemistry,Guangdong Key Laboratory of E nvironmental Resources Utilization and Protection,Guangzhou Institute of Geoche mistry,Chinese Academy of Science,Guangzhou 510640,China;2.School of Chemistry and Chemical Engineering,Northwest Normal University, Lanzhou 730070,China 3.School of Chemistry and Chemical Engineering,Sun Yat-sen University,Guan gzhou 510275,China  
The surfactants modified TiO2 pillared montmorillonites were prepare d by Sol-gel method at certain ratio of Ti(OC4H9)4 to acetic acid by using mont morillonites from different localities,such as Hebei,Lin'an and Anji,and Nei Mongol,China,and modified by cation surfactant Cetyltrimethyl ammonium bromid e (CTMAB) at the same time.Scanning electron microscopy (SEM) and X-ray diffra ction (XRD) were used to investigate the texture of prepared catalysts,and thei r BET surface areas were also measured.The results indicate that the pillared m ontmorillonites were well pillared by the anatase TiO2 and the BET surface areas were larger than the original one.The adsorption and photocatalytic performanc e of different prepared pillared clays were also studied by using methyl orange as mode organic pollutant.The pillared montmorillonites from different localiti es exhibited different adsorption and photocatalytic property which was mainly r esulted from their different compositions and interlayer structures.Moreover,i t is found that the TiO2 pillared clay by using Lin'an montmorillonite is an ex cellent photocatalyst for the degradation of mode organic pollutant.
【Fund】: 国家自然科学基金(40302013 40572173);; 广东省自然科学基金(030466);; 广东省“十五”重大科技计划项目(2005A30401001)
【CateGory Index】: O643.36
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