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《Geochimica》 2012-02
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Application of catalytic hydropyrolysis in solid bitumen-source correlation of the paleo-oil reservoirs in Nandan area

FANG Yun-xin1,2,GENG An-song1,LIAO Yu-hong1 and WU Liang-liang1,2 1.State Key Laboratory of Geochemistry,Guangzhou Institute of Geochemistry,Chinese Academy of Sciences,Guangzhou 510640,China; 2.Graduate University of Chinese Academy of Sciences,Beijing 100049,China  
The Dachang Middle-Devonian solid bitumen and its potential source rock,Devonian mudstone of trough facies in the Nandan area,south China,are all at over-mature stage.Low concentration of extractable organic matter,intense thermal alterations,and sever biodegradation may obscure the oil-source correlations based on routine biomarkers.Thus,direct molecular geochemical evidences are absent in most bitumen-source correlation studies.Catalytic hydropyrolysis is a new approach that can release biomarkers from highly mature kerogen and solid bitumen.It shows the advantages to maximize the yields of covalently-bound biomarkers from kerogen,to minimize structural rearrangement of biomarker species,and to maintain the biologically-inherited stereochemistry.In the research,the covalently-bound biomarkers and n-alkanes released from the Middle-Devonian solid bitumen and two kerogens of the potential Devonian mudstone of trough facies in the Nanpanjiang Depression by catalytic hydropyrolsis were analyzed for GC-MS and GC-IRMS to clarify the origin of organic matter in the paleo-oil reservoirs.The results indicated that the Devonian mudstone of trough facies probably were the main source for the Dachang Middle-Devonian solid bitumen in Nandan area.
【Fund】: 国家自然科学基金(40739902);; 国家油气重大专项(2011ZX 05008-002)
【CateGory Index】: P618.13
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