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《Chinese Journal of Atmospheric Sciences》 2001-02
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The Simulation and Estimation of Radiative Properties and Radiative Forcing due to Sulfate and Soot Aerosols

Zhang Lisheng and Shi Guangyu (State Key Laboratory of Numerical Modeling Atmospheric Sciences and Geophysical Fluid Dynamics, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029)  
Using complex refractive index data of sulfate and soot aerosols, the radiative properties of the aerosols from 0.2-40 um wavelength were calculated by an accurate Mie scattering algorithm. Based on the mass concentration data of aerosols simulated by LLNL CTM model and the improved aerosol parameterization in GOALS / AGCM, the radiative forcing of the global anthropogenic sulfate and soot were estimated at first time in China. The results show that: (1) The largest center of the radiative forcing due to sulfate is located at West Europe in summer, and the central value is about -5.0 W / m2; (2) The largest value of the forcing due to soot occurs in South America and South and Central Africa in summer and amounts to 4.0 W/ m2, (3) The radiative forcing caused by anthropogenic aerosols in the Southern Hemisphere cannot be ignored; (4) The radiative forcing due to human activity in some areas can be comparable in magnitude with the forcing caused by greenhouse gases, such as CO2 etc.
【Fund】: 国家“九五”重中之重!96—908—01—06专题;; 国家自然科学基金资助项目!49875012
【CateGory Index】: X513
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