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《Quaternary Sciences》 2005-05
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CHARACTERIZATION OF WATER-ROCK INTERACTION AND POLLUTION OF KARSTIC HYDROLOGICAL SYSTEM: A STUDY ON WATER CHEMISTRY AND Sr ISOTOPE OF SURFACE/GROUND WATER OF THE GUIYANG AREA

Lang Yunchao ①② Liu Congqiang ① Han Guilin ① Zhao Zhiqi ① Li Siliang ①②(①State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang 550002; ②Graduate School of the Chinese Academy of Sciences, Beijing 100039)  
The chemistry and Sr isotopic composition of surface/ground waters of the Guiyang city and its adjacent areas represent a typical hydrogeochemical signature of a typical karstic hydrological system. Dissolved load of surface and ground waters are mainly dominated by Ca 2+, Mg 2+, SO 2-_ 4 and HCO-_ 3, which are derived mainly from chemical weathering of carbonate rocks (limestone and dolomite) and dissolution of sulfate evaporates. Contribution of silicate weathering to the water system is very small. The variations of major cation co[CS]mpositions, such as Mg 2+/Ca 2+ and Sr 2+/Ca 2+ ratios, are controlled by both weathering sources and water-rock interaction. The Sr isotope compositions of the sewage samples show no significant differences with those of the surface and ground waters, and hence can not be used to trace the contaminant cycling. However, Sr isotope, when combined with chemical composition, can be a powerful tool to trace the source of contaminants. Anthropogenic inputs to the ground water system are mainly K +, Na +, Cl -, SO 2-_ 4 and NO-_ 3, among which the Na +, Cl -, SO 2-_ 4 and NO-_ 3 components can be used as the indicators of the ground water pollution. These contaminants are of higher concentrations in winter-season water, as a result of a smaller volume of water and hence smaller buffering capacity the water system. The ground waters have more NO-_ 3 than the surface water, indicating that the NO-_ 3 can be accumulated or present for a long time in the ground water system. The ground waters show co-variations in chemical composition with the surface water, and show significant differences in chemical composition in winter-[CS] and summer-season. In addition, the chemical compositions of the studied waters show a mixing of surface and ground waters. The obtained geochemical evidence demonstrates that the surface and ground water in the karstic hydrological system exchanges quickly and hence is an easily subject to impact of human activities.
【Fund】: 中国科学院知识创新工程项目(批准号:KZCX3-SW-140 KZCX2-105);; 国家自然科学基金项目(批准号:40273010 40372108)资助
【CateGory Index】: P641.3
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