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《Earth Science Frontiers》 2006-03
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Effectiveness of thermochemical sulfate reduction on oil and gas industry—a H_2S formation accelerating development of the secondary pores in reservoirs

ZHU Guang-you~(1),ZHANG Shui-chang~(1),MA Yong-sheng~(2),Liang Ying-bo~(1),GUO Tong-lou~(2),ZHOU Guo-yuan~(3)1.Research Institute of Petroleum Exploration and Development,China National Petroleum Corporation,Beijing 100083,China 2.Institute of Southern Exploration and Development Division Company of SINOPEC,Kunming 650200,China 3.East Sichuan Drilling Co.Ltd,Sichuan Petroleum Administration,Chongqing 400021,China  
Natural gas,with high contents of H_2S,is generated mainly by the important process of thermochemical sulfate reduction(TSR).During this process,and under high temperature,hydrocarbons deoxidize sulfate to acidic gases,such as H_2S and CO_2,Because of the viral and high corrosion dangers,more attention has been given to the harmful effects of H_2S in well drilling,completion,purifying processes,and in the transport in oil and gas industry.TSR and H_2S have been perceived as negative in the past and were shunned in the oil and gas exploration.Nevertheless,recent research shows that the TSR process plays an effective role in oil and gas industry.First,TSR process needs SO~(2-)_4 dissolved from sulfate,which causes the reservoir pore space to make an initial elementary improvement;secondly,the H_(2)S generated by TSR processes is dissolved in water and exhibit strong acidity,which results in the corrosion of dolostone.Under high temperature conditions and with water involved in the process,H_(2)S and dolostone give rise to a strong interaction between acidic fluid and rock(water/rock reaction).This stimulates the development of secondary pores and the formation of high-quality reservoir with high porosity and permeability.The corrosion increases the lower conservation limit of oil and gas reservoir and makes the formation of a deep natural gas reservoir possible.Nowadays,the Feixianguan formation(T_(1)f fm.) shows lower pressure coefficient and filling degree,which is related to the reservoir's dilation caused by the corrosion in the TSR process.The exploration results have proved that all the natural gas with high contents of H_2S were found in high-quality reservoirs,with sufficiently developed secondary pores,in Sichuan basin,southwest China,where the lithology is mainly dolostone.High-quality reservoirs may still be present to depths of more than 8 000 m.
【Fund】: 中国石油天然气股份公司科技项目(中国高含硫化氢天然气田资源分布与开发战略:040502-10-01);; 国家重点基础研究发展规划资助项目(2001CB209100)
【CateGory Index】: P618.13
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10 HU Zuo-wei1,HUANG Si-jing1,LI Zhi-ming2,ZHANG Xue-hua1,XUE Er-she2,LIU Tao1 1.State Key Laboratory of Oil and Gas Reservoir Geology and Exploitation,Chengdu University of Technology,Chengdu 610059,China; 2.Wuxi Institute of Petroleum Geology,SINOPEC Exploration & Production Research Institute,Wuxi 214151,China;Preliminary application of the dolomite-calcite oxygen isotope thermometer in studying the origin of dolomite in Feixianguan Formation,Northeast Sichuan,China[J];Journal of Chengdu University of Technology(Science & Technology Edition);2012-01
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1 Pan Liyin~(1,2) Liu Zhanguo~1 Li Chang~1 Shou Jianfeng~(1,2) Zhang Jianyong~(1,2) Zhang Jie~(1,2) Shen Anjiang~(1,2) Zhou Jingao~(1,2) Zheng Xingping~(1,2) 1 PetroChina Hangzhou Research Institute of Geology,Hangzhou 310023,Zhejiang 2 Key Laboratory of Carbonate Reservoir,CNPC,Hangzhou 310023,Zhejiang;Dolomitization and its relationship with reservoir development of the Lower Triassic Feixianguan Formation in eastern Sichuan Basin[A];[C];2011
2 Wu Shiqiang~1 Qian Yixiong~1 Li Huili~1 Yang Suju~2 Sha Xuguang~2 Xia Yongtao~2 Ma Qingyou~2 Zhu Xiuxiang~2 1 Research Institute of Exploration & Production,SINOPEC,Beijing 100083 2 Exploration and Development Research Institute,SINOPEC Northwest Company,Urumqi 830011,Xinjiang;Characteristics and main controlling factors of dolostone reservoir of the Middle-Lower Ordovician Yingshan Formation in Katak Uplift of Tarim Basin[A];[C];2011
3 CAI ChunFang,CAI LiuLu,ZHANG Jun,CAI XunYu and LI KaiKai 1.Key Lab of Petroleum Resources,Institute of Geology and Geophysics,Chinese Academy of Sciences,Beijing 100029,China 2.Department of Science and Technology,SINOPEC,Beijing 100728,China 3.Oilfield Department,SINOPEC,Beijing 100029,China;H_2S-generation by methane-dominated TSR and carbon isotope fractionation in Lower Triassic Feixianguan Formation,Northeast Sichuan Basin[A];[C];2013
4 LIJO Xiaorong LEI Yuhong ZHANG Likuan CHEN Ruiyin CHEN Zhankun XU Jianhua ZHAO Jian (Key Laboratory of Petroleum Resources Research,Institute of Geology & Geophysics, Chinese Academy of Sciences,Beijing 100029,China);Characterization of carrier formation for hydrocarbon migration:concepts and approaches[A];[C];2013
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