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《Journal of Fudan University(Natural Science)》 2011-04
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Degradation of Rhodamine B by High-Voltage Pulsed Dielectric Barrier Discharge in Liquid-Gas Medium

ZHAO Hai-yang1,LIU Ke-fu1,QIU Jian1,HE Jian2,HOU Hui-qi2(1.Institute of Electrical Light Sources,Fudan University,Shanghai 200433,China;2.Institute of Environmental Science,Fudan University,Shanghai 200433,China)  
A non-thermal plasma processing system was established by means of high-voltage pulsed dielectric barrier discharge in liquid-gas medium.Rhodamine B solution was chosen as the target pollutant and the degradation rates under different experimental conditions were investigated.The obtained results showed that the removal rate of Rhodamine B could be improved either by increasing the peak voltage and frequency of the pulse or by increasing the discharge time.The initial pH value of the solution had little effect on the process.For higher initial solution concentration,the degradation rate decreased,but the yield increased.Different gas introduced would influence the reaction process differently and the efficiency increased in the order of oxygen air nitrogen.Under the condition of 20kV peak pulsed voltage,250Hz pulse frequency,90mg/L initial concentration,6.4 initial pH,12.0L/min oxygen pumped in,the removal rate of Rhodamine B reached 99.1% after 12min treatment time.
【Fund】: 国家自然科学基金(11075041)资助项目
【CateGory Index】: X703
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