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《JOURNAL OF MOLECULAR CATALYSIS (CHINA)》 1999-06
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Catalyzed CO_2 Reforming of Methane to Synthesis Gas β-Alumina Type Hexaaluminate BaNiAl_(11)O_(19-δ)

XU Zhan-lin; BI Ying-li;ZHEN Kai-ji(Department of Chemistry, Jilin University, Changchun 130023)  
In this paper,β-Alumina type hexaaluminate oxides BaNiAl11O19-δ catalyst was propared by decomposition of corresponding nitrates and calcination at high temperature, in which Ni was the active component. The structure and properties of BaNiAl11O19-δ were investigated .using XRD, XPS, TPR and TGA techniques. The results showed that the re f duced hexaa1uminate BaNiAl11O19-δ exhibit significant catalytic activity and stability for CO2reforming of methane to synthesis gas at 780℃ for 18 h, the conversion of CH4 and CO2 are kept over 96. 6% and 94. 8%, respectively, the .amount of the carbon deposition is only 1. 98%. No deactivation occurs because only a litt1e carbon deposition is formed on catalysts.
【CateGory Index】: TQ426
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