Full-Text Search:
Home|Journal Papers|About CNKI|User Service|FAQ|Contact Us|中文
《Journal of Molecular Catalysis》 2007-02
Add to Favorite Get Latest Update

Surface Amino Functionalization of Mesoporous Molecular Sieve MCM-41 and Application

ZHANG Yi-ping1, 2, ZHOU Chun-hui1, FEI Jin-hua3, YU Ying-min3, ZHENG Xiao-ming3 (1. School of Chemical Engineering and Materials Science, Zhejiang University of Technology, Hangzhou 310032, China; 2. Department of Chemistry, Zhejiang Education Institute, Hangzhou 310012, China; 3. Institute of Catalysis, Xixi Campus, Zhejiang University. Hangzhou 310028, China)  
The amino-functionalized mesoporous molecular sieve was prepared by using γ-aminopropyltrimethoxysilane to react with MCM-41. The results of XRD, surface area, elemental analysis, TG, FT-IR and TEM indicated the successful tethering of organic amino group to the MCM-41 while the hexagonal structural character was mostly retained. We prepared ruthenium based catalyst supported on functionalized MCM-41, and use it to the CO2 hydrogenation to formic acid. The results indicated that the immobilized ruthenium catalyst not only overcame the disadvantage of difficult separation from the reaction system and can be reusable, but also obtained higher activity than homogeneous counterparts.
【Fund】: 浙江省自然科学基金(Y405088);; 浙江省工业催化重中之重学科开放基金资助项目.
【CateGory Index】: O643.36
Download(CAJ format) Download(PDF format)
CAJViewer7.0 supports all the CNKI file formats; AdobeReader only supports the PDF format.
【References】
Chinese Journal Full-text Database 1 Hits
1 SONG Wei-ming,DENG Qi-gang(College of Chemistry and Chemical Engineering of Qiqihar University,Qiqihar 161006,China);Preparation,characterization and catalysis performance of mesoporous composite nickel oxide[J];China Surfactant Detergent & Cosmetics;2008-06
【Citations】
Chinese Journal Full-text Database 2 Hits
1 ZHAN Wangcheng,LU Guanzhong,WANG Yanqing(Lab for Advanced Materials,Research Institute of Industrial Catalysis,East China University of Science and Technology,Shanghai 200237);Preparation and catalytic activities of functionalized mesoporous molecular sieves[J];Chemical Industry and Engineering Progress;2006-01
2 Liu Jian~ 1,2 Yang Qihua~ 1** Zhang Lei~1 Guo Yajun~2(1.Dalian Institute of Chemical Physics,Chinese Academy of Sciences,Dalian 116023,China;2.School of Chemical Engineering,Harbin Engineering University,Harbin 150001,China);Advances in Hybrid Organic-Inorganic Mesoporous Silicas[J];Progress In Chemistry;2005-05
【Co-citations】
Chinese Journal Full-text Database 9 Hits
1 ZHOU Le-zhou1,ZHOU Fang-qin1,HUANG Rong-hui1,LIU Zheng-hua1 and JIANG Fang-ming2(1.College of Chemistry,Xiangtan Univerdity,Xiangtan 411105;2.Fireworks and Firecracker Inspection Centre of Hunan Entry-Exit Inspection and Quarantine Bureau,Liuyang 410300);Study on adsorption performance of trace Hg on an organic-inorganic mesorporous material[J];Chinese Journal of Analysis Laboratory;2008-09
2 ZHANG Tao,FENG Xiu-juan*,YAN Mei,BAO Ming(State Key Laboratory of Fine Chemicals,Dalian University of Technology,Dalian 116012,China);Preparation and application of SBA-15-supported palladium catalyst for Suzuki coupling reactions in supercritical carbon dioxide[J];Journal of Molecular Science;2008-01
3 DU Li,LIU Junmin,YANG Xu,LIAO Shijun(School of Chemistry,South China University of Technology,Guangzhou 510641,Guangdong,China);Advances in mesoporous molecular sieves[J];Chemical Industry and Engineering Progress;2007-06
4 JI Yuguo1,ZHAO Zhen1,YU Changchun2,DUAN Aijun1,JIANG Guiyuan1(1State Key Laboratory of Heavy oil Processing,China University of Petroleum,Beijing 102249,China;2CNPC Key Laboratory of Catalysis,China University of Petroleum,Beijing 102249,China);Progress of cobalt-based catalysts in Fischer-Tropsch synthesis[J];Chemical Industry and Engineering Progress;2007-07
5 Zhang Xueao~(**) Liu Changli Qian Siwen Wu Xiaosen Wang Jianfang Wu Wenjian(College of Aerospace and Material Engineering,National University of Defense Technology,Changsha 410073,China);Preparation of Ordered Mesoporous Silica Thin Films and Their Assembly Chemistry[J];Progress in Chemistry;2006-10
6 Zhai Shangru~(1,2**) Wei Li~1 Yang Dongjiang~2 Wu Dong~2 Sun Yuhan~2(1.Department of Chemical Engineering and Materials,Dalian Institute of Light Industry,Dalian 116034,China;2.State Key Laboratory of Coal Conversion,Institute of Coal Chemistry,Chinese Academy of Sciences,Taiyuan 030001,China);Preparation and Applications of Silica/Aluminum-Based Micro/Mesoporous Composite Molecular Sieves[J];Progress in Chemistry;2006-10
7 Zhang Yiping~(1,2**) Zhou Chunhui~1 Wang Xuejie~2 Yang Tong~2 Xu Yuzhan~2(1.College of Chemical Engineering and Materials Science,Zhejiang University of Technology,Hangzhou 310032,China;2.Department of Chemistry,Zhejiang Education Institute,Hangzhou 310012,China);Preparation and Characterization of Organo-Functionalized Mesoporous Silica[J];Progress in Chemistry;2008-01
8 Lü YongjunLi PeijinGuo YanglongWang YanqinLu Guanzhong~(**)(Lab for Advanced Materials,Research Institute of Industrial Catalysis,East China University of Science and Technology,Shanghai 200237,China);Immobilization of Enzymes on Mesoporous Materials[J];Progress in Chemistry;2008-Z2
9 Hu Chenhui Chen Jing Quan Jicai Wang Jintang (Department of Applied Chemistry,College of Science,Nanjing University of Technology,Nanjing 210009);Research of Chiral Modification of MCM-41 and Its Catalytic Activities[J];Advances in Fine Petrochemicals;2009-01
【Co-references】
Chinese Journal Full-text Database 10 Hits
1 LI Hui-yun,WANG Wei-min (Anyang Teachers college,Anyang 455000,China);Dispersion Capacity of α-Fe_2O_3 on Mesoporous Molecular sieve MCM-41[J];JOURNAL OF AAYANG TEACHERS COLLEGE;2000-02
2 XUE Hong-yan,YIN Yan-bing,GAO Xiao-hui(College of Chemistry and Chemical Engineering of Qiqihar University,Qiqihar161006,China);Ethoxylation of fatty alcohol using lanthanum borate supported on Y-molecular sieve as catalyst[J];China Surfactant Detergent & Cosmetics;2004-06
3 YU Jianqiang 1, LI Can 1, XU Lei 2, LI Meijun 1, XIN Qin 1, LIU Zhongmin 2* (State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, The Chinese Academy of Sciences, Dalian 116023, China; 2 Dalian Institute of Chemical Physic;Synthesis of Ti-MCM-41 Using Colloidal Silica and Titanium Trichloride Ⅰ. Synthesis of Ti-MCM-41 Molecular Sieve[J];Chinese Journal of Catalysis;2001-03
4 MA Hui, HE Jing, David G EVANS, DUAN Xue * (The Key Laboratory of Science and Technology of Controllable Chemical Reactions of Ministry of Education, Beijing University of Chemical Technolgy, Beijing 100029, China);Study on Structure Design and Chemical Affinity-Selectivity of Titanium-Grafted MCM-41 Catalyst[J];Chinese Journal of Catalysis;2002-05
5 TAO Liang, YIN Donghong~*, TAN Rong, YU Ningya~*, YIN Dulin(Institute of Fine Catalysis and Synthesis, Hunan Normal University, Changsha 410081, Hunan, China);Epoxidation of Cyclohexene Catalyzed by Mn(salen) Complex in Ionic Liquids[J];Chinese Journal of Catalysis;2006-05
6 HE Leqin,ZHAO Jiquan~*,ZHANG Yaran,ZHAO Dongmin,ZHAO Shanshan(School of Chemical Engineering,Hebei University of Technology,Tianjin 300130, China);Preparation of Chiral Oligomeric Cyclic salen-Mn(Ⅲ) Complex and Its Catalytic Performance for Asymmetric Epoxidation of Olefin[J];Chinese Journal of Catalysis;2006-08
7 ZHAO Shanshan,ZHAO Jiquan,HE Leqin,LI Na,ZHAO Dongmin(School of Chemical Engineering,Hebei University of Technology,Tianjin 300130,China);Preparation of Sugar-Based Chiral Salen-Mn(Ⅲ) Complex and Its Application in Asymmetric Epoxidation[J];Chinese Journal of Catalysis;2007-07
8 GUO Rui, MA Jun, WU Nian\|zu, YANG Xi\|yao (College of Chemistry & Molecular Engineering, Peking University, Beijing 100871, China);Study of Dispersity of MoO_3 on the Surface of Mesoporous Molecular Sieve MCM-41[J];Journal of Molecular Catalysis (China);2001-05
9 XIAO Feng-Shou *, HAN Yu, QIU Shi-Lun (College of Chemistry, Jilin University, Changchun 130023, China);Acidity and Hydrothermal Stability of Mesoporous Materials[J];Chemical Research In Chinese Universities;2002-10
10 CAI Qiang, ZHANG Hui Bo , LIN Wen Yong, PANG Wen Qin * (Key Laboratory of Inorganic Synthesis & Preparative Chemistry, Jilin University, Changchun, 130023; Department of Chemical Engineering , Fushun University, Fushun, 113001);The Synthesis of Mesoporous Molecular Sieve MCM 48[J];CHEMICAL RESEARCH IN CHINESE UNIVERSITIES;1999-05
【Secondary Citations】
Chinese Journal Full-text Database 8 Hits
1 ZHANG Meiying *, WANG Lefu, HUANG Zhongtao(College of Chemical Engineering, South China University of Technology, Guangzhou 510640, Guangdong, China);Synthesis Conditions and Catalytic Performance of Hexagonal Mesoporous Silica Containing Copper[J];Chinese Journal of Catalysis;2003-12
2 SHEN Bao-jian~*, REN Shen-yong, GUO Qiao-xiaoalysis of CNPC, University of Petroleum, Beijing 102249, China);Covalent Grafting of Zirconocene Dichloride Moiety on MCM-41[J];Journal of Molecular Catalysis;2004-02
3 WANG Ya Jun 1, TANG Yi 1* , WANG Xing Dong 1, YANG Wu Li 2 NI Zheng 1, HUA Wei Ming 1, YUE Ying Hong 1, GAO Zi 1 [WT5”BX](1. Department of Chemistry, 2. Department of Macromolecular Science, Fudan University, Shanghai 200433, China);Synthesis of Silicate Materials with Micro/Macroporous Bimodal Pore Systems[J];CHEMICAL RESEARCH IN CHINESE UNIVERSITIES;2000-07
4 WANG Run-Wei,HU Lei,CHU Bin,ZHU Guang-Shan,QIU Shi-Lun * (State Key Laboratory of Inorganic Synthesis and Preparative Chemistry,College of Chemistry, Jilin University,Changchun 130023,China);Synthesis,Characterization and Catalytic Properties of Mesoporous Materials with Loading of TS-1 Precursors[J];Chemical Research In Chinese Universities;2004-08
5 GUO Jianwei 1, WANG Lefu 2,CUI Yingde 3 and LIU Sa 2 ( 1Faculty of Chemical Engineering & Light Industry,Guangdong University of Technology,Guangzhou 510090,Guangdong,China; 2South China University of Technology, Guangzhou 510640,Guangdong,China; 3Zhongkai Agrotechnical College,Guangzhou 510225,Guangdong,China);SYNTHESIS OF Ti-MCM-41 MOLECULAR SIEVES BY ELECTROSTATIC S~+X~-I~+ ASSEMBLY PATHWAY AND ITS CATALYTIC OXIDATION PERFORMANCE[J];Journal of Chemical Industry and Engineering(China);2004-07
6 LI Ping 1, ZHAO Yue 2, LU Guan zhong 1* , ZHAO Xiu ge, LU Wen zhi 2, XIAO Wen de 2 (1.Research Institute of Industrial Catalysis ECUST, Shanghai 200237, China; 2. Research Center of Chemical Reaction Engineering ECUST);Effect of SO_2 on NO Catalytic Oxidation I. Role of Supports[J];Journal of East China University of Science and Technology;2002-04
7 JIA, Xue-Ping YANG, Chun (College of Chemistry and Environmental Science, Nanjing Normal University, Nanjing 210097);Characterization of Surface Functionalised Mesoporous Molecular Sieve SBA-3[J];Acta Chimica Sinica;2002-09
8 ZHAI, Shang-Ru ZHANG, Ye WU, Dong SUN, Yu-Han  (State Key Laboratory of Coal Conversion, Institute of Coal Chemistry, Chinese Academy of Sciences, Taiyuan 030001);Efficient Synthesis of Mesoporous MCM-48 by Using Mixed Surfactants and pH Adjustment Method[J];Acta Chimica Sinica;2003-03
©2006 Tsinghua Tongfang Knowledge Network Technology Co., Ltd.(Beijing)(TTKN) All rights reserved