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《Chemical Research In Chinese Universities》 2002-04
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Studies on Selectively Catalytic Reduction of NOxby Methane over Ag-ZSM-5 Catalysts

SHI Chuan, CHENG Mo-Jie, QU Zhen-Ping, YANG Xue-Feng, BAO Xin-He(State Key Laboratory of Catalysis, Dolian Institute of Chemical Physics, Chinese Academy of Sciences,Dalian 116023, China; 2. Laboratory of Plasma Physical Chemistry,Dalian University of Tec  
Ag-ZSM-5 catalysts were investigated for the selectively catalytic reduction of NO by methanein the excess of oxygen. The adsorption properties of NOx and the reaction of absorbed NOx with CH4 werestudied through TPD and TPSR measurements. NOx was effectively and selectively reduced by CH4 overAg-ZSM-5 catalysts. The co-adsorption of NO and O2 over Ag-ZSM-5 catalyst led to the formation of ad-sorbed NO3 species, which could be effectively reduced by CH4. Even in the presence of O2, NO3 specieswere more reactive than O2. The priority of CH4 reaction with surface NO3-species to form N2 was clearlyobserved.
【Fund】: 国家自然科学基金(批准号:20003011)和“973”计划资助.
【CateGory Index】: O643.3
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