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《Chemical Research In Chinese Universities》 2005-12
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Fenton Photocatalytic Degradation of Organic Dye Under Visible Irradiation

HUANG Ying-Ping~(1*),LIU De-Fu~(1),ZHANG Shui-Ying~(1),ZHANG De-Li~(1),MA Wan-Hong~(2),ZHAO Jin-Cai~(2) (1.Research Center for Eco-environmental Sciences,China Three Gorges University,Yichang 443002,China;2.Research Center of Molecule Sciences,Institute of Chemistry,Chinese Academy of Sciences,Beijing 100080,China)  
A photooxidative system for degradation of organic dye pollutant RhB as an objective compound was reported under visible irradiation(λ450 nm) by using Fe~(3+)/H_(2)O_(2) as the Fenton reagent. It was found that,in the system with pH3.0,visible light irradiation significantly accelerates the degradation process by photosensitive effect.After 160 min the RhB was mineralized with a yield of 71.8%.Bromocresol green reaction spectrophotometrically,spin-trapping electron paramagnetic resonance,UV-Vis spectroscopy,IR and total organic carbon(TOC) measurements were used to detect the photoreaction process.The photocatalytic degradation pathway mainly involves the formation of()~·OH and carboxylie acids are the main intermediate products. H_2O_2 of Fe~3+/H_2O_2/RhB system was utilized lowlier than that of supermolecular metal/organie complexes or supported catalysts system.
【Fund】: 国家自然科学基金(批准号:20373074);; 国家重点基础研究发展计划(批准号:2003CB415006-3);; 湖北省高层次人才基金资助
【CateGory Index】: X703
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