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《Chemical Research In Chinese Universities》 2005-12
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IR Spectroscopic Study on Selective Adsorption of Sulfur-containing Compounds from Gasoline Distillation on Copper-exchanged Y Zeolite

TIAN Fu-Ping~(1,2),WU Wei-Cheng~(2),JIANG Zong-Xuan~(2),YANG Yong-Xing~(2),CAI Tian-Xi~(1),LI Can~(2*)(1.State Key Laboratory of Fine Chemicals,Dalian University of Technology,Dalian 116012,China;2.State Key Laboratory of Catalysis,Dalian Institute of Chemical Physics,Chinese Academy of Sciences,Dalian 116023,China)  
Desulfurization of gasoline distillation with adsorption was studied at ambient temperature and pressure by using CuNaY(NaY exchanged with copper nitrate aqueous solution) as the adsorbents.The gasoline distillation was composed of thiophene-cyclohexane solution(115.0 μg/mL) with or without toluene.For the solution without toluene,no detectable sulfur was found in the effluent when the effluent volume was less than 40 mL,while the addition of toluene resulted in an evident drop of the adsorption performance for(CuNaY.) FTIR spectra indicate that the conversion of Cu~(2+) to Cu~(+) took place during the pretreatment of(CuNaY) adsorbent,and the interaction mode between the adsorbed thiophene molecules and Cu~(+) is π complexation.This adsorption mode is easily affected by aromatic compounds,resulting in the significant decrease of adsorption capacity in model gasoline containing toluene on CuNaY.
【Fund】: 国家“九七三”计划项目(批准号:G2000048003)资助
【CateGory Index】: TE622.1
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