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《Spectroscopy and Spectral Analysis》 2012-05
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Study of Ice Ⅶ Structure Influenced by High Pressure Using Raman Spectrum

JIA Li-hua1,2,WANG Yi-ding2,MEN Zhi-wei3,QU Guan-nan3,LI Zuo-wei1*,HE Li-qiao3* 1.State Key Laboratory of Superhard Materials,Jilin University,Changchun 130012,China 2.College of Electronic Science and Engineering,Jilin University,Changchun 130012,China 3.College of Physics,Jilin University,Changchun 130012,China  
Raman spectra of ice Ⅶ phase were obtained at room temperature when the pressure was from 2.5 to 23 GPa.The experimental results indicate that the oxygen atoms distance do-o of ice decreased with pressure increasing,which results in that hydrogen bond is shortened,O—H bond is lengthened,force constant is reduced,and Raman spectra are red shifted.The orientation order of proton(hydrogen atom) is first increased and then decreased with varying the pressure,which leads to the Raman intensity increasing and then decreasing,and Raman linewidth is decreased and then increased,and the linewidth is the least when the pressure is 13 GPa.
【Fund】: 国家自然科学基金项目(10974067 11104106);; 吉林省科技厅项目(20101508 201101037 201115033);; 中国博士后科学基金面上项目(20100481062);; 吉林大学研究生创新项目(20111025)资助
【CateGory Index】: O433.4
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