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《Industrial Catalysis》 2004-11
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Latest advances in the catalysts for synthesis of DMCby liquid-phase oxidative carbonylation of methanol

ZHANG Xiao-bing~(1,2), LI Zhong~1, WEI You-cun~2 Shanxi Province, Taiyuan University of Technology, Shanxi Taiyuan 030024, China; 2. Technological Center of Taiyuan Coal Gasification (Group) Co. Ltd, Shanxi Taiyuan 030024, China)  
Current DMC (dimethyl carbonate) synthesis catalysts for liquid-phase oxidative carbonylation of methanol include four catalytic systems, i. e., Cu, Co, Pd-Cu and Se systems, among which CuCl catalyst has been commercialized. Current problems with CuCl catalyst include deterioration of the activity due to loss of Cl~- and equipment corrosion. The problems are usually solved by stabilization of Ci~- via introducing ligands or additives, or replacing the Cl~- by other anions. The latter shows more promising prospect for commercial application.
【Fund】: 山西省归国留学基金(200331);; 山西省自然科学基金(20031022)
【CateGory Index】: TQ225.242;TQ42
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