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《Chemical Industry and Engineering Progress》 2019-06
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Research progress on the electrochemical storage mechanisms of metalorganic frameworks in secondary batteries

DENG Qijiu;FENG Shuaishuai;TIAN Congcong;HUI Peng;YAN Yinglin;YANG Rong;School of Materials Science and Engineering, Xi'an University of Technology;School of Science, Xi'an University of Technology;  
Metal organic frameworks(MOFs) with well-developed porosity, large specific surface area,controllable structure and functionalities have been widely used as electrode materials in secondary batteries. In this paper, the mechanisms of MOFs in secondary-ion batteries have been systematically reviewed in terms of the metal center and organic ligands, including conversion reaction, insert/de-insert mechanism, surface absorption/desorption mechanism. And the energy storage characteristics of various mechanisms and their impact on the electrochemical performance are also analyzed. Additionally, the potential applications of MOFs in secondary-ion batteries based on sodium-ion and potassium-ion with larger radius are also addressed. Finally, the structural design and development trend of an ideal MOFsbased electrode material are briefly outlined. Stable metal ions with abundant energy storage sites should be used as organic ligand conjunction.
【Fund】: 中国博士后面上项目(2018M633544);; 西安理工大学博士启动基金(101-451117007);; 国家国际科技合作专项项目(2015DFR50350);; 国家自然科学基金(51702256);; 陕西省科技计划(2017JQ5055);; 陕西省自然科学基础研究计划(2017GY-160)
【CateGory Index】: O641.4;TM912
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