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《Journal of Chemical Industry and Engineering(China)》 2004-12
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PREPARATION OF MCM-22 ZEOLITE PELLETS BY VPT METHOD AND ALKYLATION CATALYTIC PERFORMANCE

LI Yingxia, CHEN Biaohua,MU Zhijun,LI Chengyue and WANG Wenxing (The Key Laboratory of Controllable Chemical Reactions of Ministry of Education, Beijing University of Chemical Technology, Beijing 100029, China)  
The vapor-phase -transport (VPT) method was adopted to prepare the grainy MCM-22 zeolite catalyst. Its physical and textural properties were characterized with XRD,SEM and BET.The catalytic performance of the catalyst was evaluated in a liquid-solid fixed bed reactor for the alkylation of benzene with propylene as a model reaction system.It was found that the MCM-22 zeolite catalyst prepared by the VPT method not only showed good crystallinity and high BET surface area, but also better crystal growth orientation and denser structure.The catalyst showed high activity, selectivity and good stability for alkylation of benzene with propylene, especially better selectivity to the end product cumene.The shaped MCM-22 zeolite catalyst prepared by the VPT method has good prospect of industrial application in synthesis of cumene.
【Fund】: 国家重点基础研究发展规划项目(No G2 0 0 0 0 480 0 6);; 中国石油化工股份有限公司项目(No X5 0 3 0 11)~~
【CateGory Index】: O643
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