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《Chinese Journal of Environmental Engineering》 2016-12
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Properties and characterization of Cu_xFe_(1-x)@γ-Al_2O_3 catalysts on treating ceramic printing wastewater with catalytic wet oxidation method

ZHOU Yanbo;ZHU Jujian;DAI Shujuan;ZHANG Yongli;School of Mining Engineering,University of Science and Technology Liaoning;School of Chemical and Environmental Engineering,Hanshan Normal University;  
Four catalysts( CuxFe1-x@ γ-Al_2O_3) were prepared using the impregnation method at room temperature,and then applied to treating ceramic printing wastewater with the catalytic wet oxidation method. Experiments were conducted on the impact of composition of the CuxFe1-x@ γ-Al_2O_3 catalyst on wet oxidation activity and stability. The results showed that the Cu0. 5Fe0. 5@ γ-Al_2O_3 catalyst displayed the highest catalytic activity and stability of the four prepared catalysts( Cu0. 5Fe0. 5@ γ-Al_2O_3,Cu@ γ-Al_2O_3,Fe@ γ-Al_2O_3 and γ-Al_2O_3).For the Cu0. 5Fe0. 5@ γ-Al_2O_3 catalyst,iron drives copper to enter the lattices of the γ-Al_2O_3 support and to form a stable solid solution( Al2 Cu O4). Therefore,this catalyst displayed the greatest hardness and stability of the four samples. After being applied for catalytic wet oxidation,the catalyst showed little change in its morphology or crystal phase,which confirmed the stability of the catalyst. Under optimal running conditions,the COD and chromaticity of the ceramic printing wastewater treated by catalytic wet oxidation method,with the catalyst CuxFe1-x@ γ-Al_2O_3,were 280 mg·L~(-1)and 20 times,respectively,which met the third emission standard on dye wastewater,under the Integrated Wastewater Discharge Standard( GB 8978-1996).
【Fund】: 辽宁省工业特种资源行业高新技术研发项目(MYF2012-23);; 2014韩山师范学院教授启动项目(QD20140615)
【CateGory Index】: X781.5
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【Citations】
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1 Zhang Hao;Cao Xianlei;Tang Gang;Liu Ying;School of Civil Engineering and Architecture,Anhui University of Technology;;Multivariate nonlinear regression analysis for preparation of Cu-Ce/TiO_2 based on orthogonal experimental design[J];环境工程学报;2015-07
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4 Zhang Yongli1 Wei Chaohai1 Luo Danping2 Chen Weilin2 Huang Zhizhen2 Yang Liushan2(1.College of Environmental Science and Engineering,South China University of Technology,Guangzhou 510006,China; 2.Department of Chemistry,Hanshan Normal University,Chaozhou 521041,China);Coagulant and processing conditions of ceramic printing wastewater treatment[J];环境工程学报;2012-12
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1 ZHOU Yanbo;ZHU Jujian;DAI Shujuan;ZHANG Yongli;School of Mining Engineering,University of Science and Technology Liaoning;School of Chemical and Environmental Engineering,Hanshan Normal University;;Properties and characterization of Cu_xFe_(1-x)@γ-Al_2O_3 catalysts on treating ceramic printing wastewater with catalytic wet oxidation method[J];环境工程学报;2016-12
2 Yongli Zhang;Feng Peng;Yanbo Zhou;School of Chemistry and Chemical Engineering, South China University of Technology;School of Chemical and Environmental Engineering, Hanshan Normal University;;Structure, characterization, and dynamic performance of a wet air oxidation catalyst Cu–Fe–La/γ-Al_2O_3[J];Chinese Journal of Chemical Engineering;2016-09
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8 YANG Shaoxia a, b , ZHU Wanpeng b , and WANG Xingang a a National Engineering Laboratory for Biomass Power Generation Equipment, School of Renewable Energy, North China Electric Power University, Beijing 102206, China b Department of Environmental Science and Engineering, Tsinghua University, Beijing 100084, China;Influence of the structure of TiO_2 , CeO_2 , and CeO_2-TiO_2 supports on the activity of Ru catalysts in the catalytic wet air oxidation of acetic acid[J];Rare Metals;2011-05
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