Full-Text Search:
Home|Journal Papers|About CNKI|User Service|FAQ|Contact Us|中文
《Environmental Science》 2014-06
Add to Favorite Get Latest Update

Contamination and Source of Polycyclic Aromatic Hydrocarbons in Epikarst Spring Water

SUN Yu-chuan;SHEN Li-cheng;YUAN Dao-xian;Key Laboratory of Eco-Environments in Three Gorges Reservoir Region,Ministry of Education,School of Geographical Sciences,Southwest University;Key Laboratory of Karst Dynamics,Ministry of Land and Resources,Institute of Karst Geology,Chinese Academy of Geological Sciences;  
The water samples were collected from four typical epikarst springs in Nanchuan District,Chongqing Municipality between October 2010 and October 2011. Sixteen priority polycyclic aromatic hydrocarbons in epikarst spring waters were quantitatively analyzed by the gas chromatography-mass spectrometer( GC-MS). The objectives of this study were to investigate the seasonal variations of polycyclic aromatic hydrocarbons' concentration,composition,source and contamination characterization in epikarst springs water. The results showed that the detection ratios of 16 PAHs in four springs were 100%. The total concentrations of 16 PAHs fluctuated greatly in epikarst spring water during one year observation,and the concentration ranged from 341 to 4 968 ng·L-1,with a mean value of1 772 ng·L-1. The total concentrations of 7 carcinogenic PAHs in rain season were all higher than those in dry season in four epikarst springs. The PAHs profiles were dominated by( 2-3) rings PAHs in spring water,which accounted for more than 50% of 16 PAHs.The PAHs in spring water mainly originated from the combustion of coal,biomass and petroleum,and during June to October 2011,PAHs originated from the combustion of coal and biomass had a larger contribution. The ratios of Ant /( Ant + Phe) and Fla /( Fla +Pyr) changing with seasons showed that Ant,Phe,Fla and Pyr were easy to migrate in epikarst soils. In 4 isomeric ratios,the ratios of Fla /( Fla + Pyr) were more sensitive to reflect the information of sources. Compared to other areas in the world,the concentration of 16PAHs in epikarst spring water is at a higher level,which shows the epikarst spring water has been suffered the PAHs pollution.
【Fund】: 中央高校基本科研业务费专项(XDJK2013B021);; 西南大学博士基金项目(SWU110258);; 应对全球气候变化地质调查综合研究项目(12120113006700);; 重庆市科委院士专项(cstc2013jcyjys20001)
【CateGory Index】: X523
Download(CAJ format) Download(PDF format)
CAJViewer7.0 supports all the CNKI file formats; AdobeReader only supports the PDF format.
【Citations】
Chinese Journal Full-text Database 10 Hits
1 CUI Xue-hui~1,LI Bing-hua~2,CHEN Hong-han~2(1.Mathematical Department,China University of Petroleum,Beijing 102249,China;2.Beijing Key Laboratory for Water Resources and Environmental Engineering,China University of Geosciences,Beijing 100083,China);Contamination Characteristics and Pollutant Sources Analysis on PAHs in Shallow Groundwater in Suburb of Taihu Plain[J];Environmental Science;2008-07
2 WANG Ying-hui~1,2,QI Shi-hua~2,YUAN Dao-xian~2,LI Jie~2,XING Xin-li~2(1.School of Environment Studies,Guangxi University,Nanning 530004,China;2.Key Laboratory of Biogeology and Environmental Geology of Ministry of Education,China University of Geosciences,Wuhan 430074,China);Distribution Character of Polycyclic Aromatic Hydrocarbons in Soils from the Karst Cavity,Guilin City,South China[J];Environmental Science;2009-05
3 HE Jiang-tao,JIN Ai-fang,CHEN Su-nuan,WEI Yong-xia(School of Water Resources and Environment,China University of Geosciences,Beijing 100083,China);Distribution of Polycyclic Aromatic Hydrocarbons in Soil Profiles in Southeast Suburb of Beijing Wastewater Irrigation Area[J];Environmental Science;2009-05
4 KONG Xiang-sheng1,2,3,QI Shi-hua1,Oramah I T1,ZHANG Yuan1,HE Shi-yi2(1.Key Laboratory of Biogeology and Environmental Geology,Ministry of Education,China University of Geoscience,Wuhan 430074,China;2.Institute of Karst Geology,Chinese Academy of Geological Science,Guilin 541004,China;3.Key Open Laboratory of Karst Ecosystem and Rocky Desertification Control,Chinese Academy of Geological Science,Guilin 541004,China);Contamination of Polycyclic Aromatic Hydrocarbons in Surface Water in Underground River of Dashiwei Tiankeng Group in Karst Area,Guangxi[J];Environmental Science;2011-04
5 LUO Qing1,SUN Li-na1 *,ZHANG Yao-hua2(1.Key Laboratory of Regional Environment and Eco-Remediation of Ministry of Education,Shenyang University,Shenyang 110044,China;2.Liaoning Acadeny of Geology and Mineral Resources,Shanyang 110032,China);Health Risk Assessment of Polycyclic Aromatic Hydrocarbons in Groundwater from Xihe River Area,China[J];Journal of Agro-Environment Science;2011-05
6 KONG Xiang-sheng1,2,3,QI Shi-hua2,JIANG Zhong-cheng1,3,HUANG Bao-jian1(1.Institute of Karst Geology,Chinese Academy of Geological Science,Guilin 541004,China;2.School of Environmental Studies,China University of Geoscience,Wuhan 430074,China;3.Key Open Laboratory of Karst Ecosystem and Rocky Desertification Control,Chinese Academy of Geological Science,Guilin 541004,China);Environmental Factors on Distribution of Polycyclic Aromatic Hydrocarbons in Soils from Dashiwei Karst Giant Doline(Tiankeng) in Guangxi,China[J];Environmental Science;2012-11
7 GAO Yan-fang,SHEN Li-cheng,YANG Ping-heng (School of Geographical Sciences,Southwest University,Beibei,Chongqing 400715,China);Research on Nitrogen pollution sources of groundwater in Chongqing Jinfo Mt.[J];Journal of Water Resources and Water Engineering;2007-06
8 YUAN Dao-xian (Institute of Karst Geology, CAGS, Karst dynamics Laboratory, MLR, Guilin 541004, China);ASPECTS ON THE NEW ROUND LAND AND RESOURCES SURVEY IN KARST ROCK DESERTIFICATION AREAS OF SOUTH CHINA[J];CARSOLOGICA SINICA;2000-02
9 LIANG Xiaoping, ZHU Zhiwei, LIANG Bin, GUAN Bizhu, ZOU Shengzhang (Institute of Karst Geology, CAGS, Guilin, Guangxi 541004,China);PRELIMINARY ANALYSIS ON HYDROGEOCHEMICAL CHARACTERISTICS OF THE EPIKARST ZONE IN LUOTA, HUNAN[J];Carsologica Sinica;2003-02
10 QIN Xiao-qun,JIANG Zhong-cheng(Institute of Karst Geology,CAGS,Guilin,Guangxi 541004,China);A REVIEW ON RECENT ADVANCES AND PERSPECTIVE IN EPIKARST WATER STUDY[J];Carsologica Sinica;2005-03
【Co-citations】
Chinese Journal Full-text Database 10 Hits
1 LIU Li-yan et al(School of Resources and Environmental Engineering,Guizhou University,Guiyang,Guizhou 550003);Preliminary Study on Optimal Models of Landscape Ecology Sustainable Development in Karst Mountainous Rural Area of Guizhou Province[J];Journal of Anhui Agricultural Sciences;2007-08
2 ZHOU Yun et al(Forestry Bureau of Bijie City,Bijie,Guizhou 551700);Discussion on the Prevention Measure of Karst Rocky Desertification in Bijie City[J];Journal of Anhui Agricultural Sciences;2008-06
3 LI Ying-gang et al (School of Geography Sciences,Southwest University,Chongqing 400715);Analysis of Karst Rocky Desertification Actuality and Sensitivity in Nanchuan of Chongqing Based on RS and GIS[J];Journal of Anhui Agricultural Sciences;2009-05
4 HUAN Huan et al (Research Institute of Water Sciences,Beijing Normal University,Beijing 100875);Discussion on the Utilization of Groundwater in Coastal Areas with Heavy Rain[J];Journal of Anhui Agricultural Sciences;2011-01
5 LI Yong-xin(School of Earth Science and Resources,China University of Geosciences,Beijing 100083);Effects of Algae in Tufa Landscape in Huanglong Scenic Area[J];Journal of Anhui Agricultural Sciences;2011-09
6 ZHANG Yuan-hai et al(Institute of Karst Geology,Chinese Academy of Geological Sciences,Guilin,Guangxi 541004);Analysis on Dashiwei Karst Characteristics and Natural Heritage Values in Leye County,Guangxi Province[J];Journal of Anhui Agricultural Sciences;2012-08
7 Cao Huan1,Su Weici2,3,Fan Xinrui1(1.Resources and Environment College of Guizhou University,Guiyang 550003,China;2.Research Institute of Mountain Resources,Guizhou Academy of Sciences,Guiyang 550001,China;3.Geography College of Chongqing Normal University,Chongqing 400047,China;);A Preliminary Discussion on the Karst of Ecosystem Health Factors and Evaluation——A Case Study in Bijie[J];Environmental Science and Management;2008-10
8 YANG Xiaoyan YUAN Renmao (Department of Urban and Enviornmental Sciences,Peking University,Beijing,100871)CHEN Suozhong (College of Geographic Sciences,Nanjing Normal University,Nanjing,210018);The Study of the Causes of Karst Collapses in Qixiashan Hill Area of Nanjing[J];Acta Scicentiarum Naturalum Universitis Pekinesis;2001-06
9 ZHANG Jia-gui~(1,2) (1.Institute of Geomechanics, Chinese Academy of Geological Sciences, Beijing100081,China; 2. China Institute of Geo-Environmental Monitoring, Beijing100081,China);Mechanism of landform control over karstification in mud limestone area along valley slope zone A case study from Three Gorges region[J];Journal of Jiling University (Earth Science Edition);2004-03
10 DONG Gui-ming1,SHU Long-cang2,TIAN Juan3,JI Ye-fei21.The School of Resource and Earth Science,China University of Mining and Technology,Xuzhou 222116,Jiangsu,China2.State Key Laboratory of Hydrology-Water Resources and Hydraulic Engineering,Hohai University,Nanjing 210098,China3.City and Environment College,Xuzhou Normal University,Xuzhou 222116,Jiangsu,China;Numerical Model of Groundwater Flow in Karst Underground River System,Southwestern China[J];Journal of Jilin University(Earth Science Edition);2011-04
【Secondary Citations】
Chinese Journal Full-text Database 10 Hits
1 DONG Bin-fang et al(College of Geography Science,Southwest University,Chongqing 400715);Effect of the Plant Root System on Preferential Flow in Soil[J];Journal of Anhui Agricultural Sciences;2006-23
2 ZHAN Hui-ying~(1,2), YUAN Jian-mei~1, JIANG Yu-feng~1, CHEN Hui~1 (1 College of Chemistry and Chemical Engineering, Northwest Normal University, Lanzhou 730070, China; 2 College of Science and Engineering, Gansu Coalesced University, Lanzhou 730000, China);Sorption isotherms and sorption thermo- dynamics of phenanthrene and naphthalene on loess soil[J];Journal of Safety and Environment;2004-04
3 CAO Jian-sheng;ZHANG Wan-jun;LIU Chang-ming;YANG Yong-hui.Institute of Genetics and Developmental Biology,Chinese Academy of Sciences,Shijiazhuang,050021,P.R.China.;Fractured rock seepage characteristics and its impact on slope stability.[J];Journal of Beijing Forestry University;2007-04
4 WANG Xi-long 1,XU Fu-liu 1,LI Ben-gang 1,CAO Jun 1,TAO Shu 1,SHEN Wei-ran 2,ZHAO Xi-mei 2 (1.Department of Urban and Environmental Sciences, Peking University, Beijing 100871,China; 2.Tianjin Environmental Protection Bureau,Tianjin 300191,China);Risk Assessment of Ecotoxicity of Benzo(a)pyrene, Fluorethene and Phenanthrene in Tianjin Wastewater Irrigated Area[J];Urban Environment & Urban Ecology;2002-04
5 ZOU Sheng-zhang, LIANG Bin, ZHU Zhi-wei, LIANG Xiao-ping (Institute of Karst Geology,The Chinese Academy of Geological Sciences,Guilin 541004, China);EFFECT OF ECOSYSTEM ON WATER RESOURCE IN KARST AREA ——A CASE STUDY IN WEST HUNAN[J];Resources and Environment in the Yangtze Basin;2004-06
6 GE Cheng-jun~1,2,AN Qiong~1,DONG Yuan-hua~1,YU Hua-mei~2(1.Institute of Soil Science,The Chinese Academy of Sciences,Nanjing 210008,China;2.South China University of Tropical Agriculture,Danzhou 571737,China);DISTRIBUTION OF ORGANIC POLLUTANTS IN AGRICULTURAL SOIL IN NANJING CITY[J];Resources and Environment in the Yangtze Basin;2006-03
7 LI Xiu-cang1,2,HU Shun-jun1,3,LI Yue-tan1,4,LI Xue-mei1,2(1.Xinjiang Institute of Ecology and Geography,Chinese Academy of Sciences,Urumqi 830011,China;2.Graduate School,Chinese Academy of Sciences,Beijing 100039,China;3.Key Laboratory for Agricultural Soil and Water Engineering in Arid Area of Education Ministry,Yangling 712100,China;4.College of Resources Science and Technology,Beijing Normal University,Beijing 100873,China);Study on the root distribution and soil water dynamics under Phragmites arid area[J];Acta Prataculturae Sinica;2008-02
8 YU Xiu-yan,DING Yong-sheng(Environmental Science & Eng.College, Dalian Maritime Univ., Dalian 116026,China);Advances of studies on the enviromental distribution of polycyclic aromatic hydrocarbons and its bioremediation[J];Journal of Dalian Maritime University;2004-04
9 ZHANG Zhi-Huan~(1,2),WANG Xue-Jun~1,TAO Shu~1,PENG Zheng-Qiong~2,CUI Yan-Hong~1,WU Shui-Ping~1,YE Bi-Xiong~2,YUAN Jin-Peng~2Hydrocarbon Accumulation, Ministry of Education; Faculty of Natural Resources & Information Technology, University of Petroleum, Beijing 102200);Vertical Distribution Characteristics of Polycyclic Aromatic Hydrocarbon Compounds from Various Soil Profiles of Tianjin[J];Scientia Geographica Sinica;2004-05
10 LI Si-liang 1,2 ,LIU Cong-qiang 1 ,XIAO Hua-yun 1 ,TAO Fa-xiang 1 ,LANG Yun-chao 1,2 ,HAN Gui-lin 1 1.State Key Laboratory of Environment al Geochemistry,Institute of Geoch emistry,Chinese Academy of Science s,Guiyang550002,China;2.Graduate School of the Chinese Academy of Sciences,Beijing100039,China;Usingδ~(15)N to assess groundwater nitrogen pol lution in Guiyang[J];Geochimica;2005-03
©2006 Tsinghua Tongfang Knowledge Network Technology Co., Ltd.(Beijing)(TTKN) All rights reserved