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《Acta Scientiae Circumstantiae》 2004-06
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Heterogeneous UV/ Fe-Cu-Mn-Y/H_2O_2 catalyst catalytic degradation of 4BS

ZHENG Zhanwang~1,LEI Lecheng~1 ,ZHANG Zheng~1,CEN Peilin~2 (Department of Environmental Engineering, Zhejiang University, Hangzhou310027; Department of Bioengineering, Zhejiang University, Hangzhou310027)  
The homogeneous UV/Fenton system's pH had to be adjusted to a limited range (3~5) and the Photo-Fenton process requires recovery of iron, so operation cost in chemicals and labor has to be added. In order to widen the application of Fenton-type oxidation processes, these drawbacks have to be overcomed by immobilization of ferric ion. Investigations showed that other transition metal ions, due to their variety of valence could replace ferric ion and serve as a like-Fenton reagent. Furthermore, different kinds of transition metal ions and their ratio in the UV/like-Fenton process will favorably affect the degradation of contamination significantly. In this article, the heterogeneous Fe-Cu-Mn-Y catalyst was developed by immobilizing Fe~(2+), Cu~(2+), Mn~(2+) on Na-Y zeolite. The degradation of 4BS has been investigated by the heterogeneous UV/Fe-Cu-Mn-Y/H_2O_2 process. The results indicated that the heterogeneous UV/ Fe-Cu-Mn-Y/H_2O_2 process shows high proficiency in catalytic oxidizing 4BS, whose 4BS removal rate reached 93.7% when the reaction time is 20 min under the standard experimental conditions (as defined in the article). Deferent from the homogeneous one, the heterogeneous process remains higher efficiency of removal of COD_(Cr) and 4BS, even in alkaline solution (pH reached 10.5). Kinetic model was correlated, which could provide the direction of the practical treatment of such deep color dye effluents.
【Fund】: 国家自然科学基金资助课题(20176053)
【CateGory Index】: X703.1
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