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《Acta Mineralogica Sinica》 2003-03
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COMPARATIVE STUDY ON THE AGGREGATION OF DIFFERENT LONG-CHAIN ALKYLAMMONIA IN MONTMORILLONTTE

ZHU Jian-xi,HE Hong-ping,GUO Jiu-gao,YANG Dan,XIE Xian-de (Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China)  
The orientation of quaternary ammonium cation in the interlayer of organic pillared montmorillonite prepared at different concentrations of DDTMAB, TDTMAB, HDTMAB has been studied using X-ray powder diffraction (XRD). The arrangement model and transmutation of DDTMA+ , TDTMA+ and HDTMA+ in the interlayer of montmorillonite were different. The arrangement model of DDTMA+ in the interlayer of montmorillonite changes in the order of lateral-monolayer →lateral-bilayer→pseudotrilayer; TDTMA+ changes in the order of lateral-monolayer →lateral-bilayer → paraffin-type monolayer→random stacking + lateral-bilayer, and HDTMA+ changes in the order of lateral-monolayer→lateral-bilayer →paraffin-type monolayer →pseudotrilayer →paraffin-type-bilayer. These differences are mainly due to the difference in length of alky chain.
【Fund】: 国家自然科学基金(批准号:49972018);; 广东省自然科学基金(批准号:990522)
【CateGory Index】: P578
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