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《Acta Physico-chimica Sinica》 2004-12
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Synergistic Effect of Eu~(3+)and Si~(4+)Co doping on Photocatalytic Activity of Titanium Dioxide

Li Yue Xiang1,2 Wang Tian Hui1 Peng Shao Qin1 LüGong Xuan2 Li Shu Ben2 (1Department of Chemistry, Nanchang University, Nanchang 330047; 2State Key Laboratory for Oxo Synthesis and Selective Oxidation,Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou 730000)  
Eu/Ti/Si composite photocatalysts were prepared by sol gel soaking process and characterized by XRD, FT IR and EPR. It has been shown that the particle diameter of Eu/Ti/Si photocatalysts decreased, the crystal transformation of titania from anatase to rutile was prevented, and the incorporation of Si4+into the matrix of the TiO2 was promoted owing to the co doping of Si4+and Eu3+. As a model reaction, the photocatalytic degradation of methyl orange was investigated. The adsorption constants of methyl orange over catalysts were evaluated and the adsorption mechanism was also discussed. Optimal doping amounts for Si4+and Eu3+are =39.06%and wEu=0.03%respectively, and the co doping of them shows a synergistic effect for photocatalytic activity of titanium dioxide. Relation between photocatalytic activity and property of the photocatalyst was discuused.
【Fund】: 国家重点基础研究发展规划项目(973)(2003CB214503);; 江西省自然科学基金(0220007);; 南昌大学“十五”“211”重点学科建设项目资助~~
【CateGory Index】: O643
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