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《Acta Scientiarum Naturalium Universitatis Pekinensis》 2015-04
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In-situ Simulation Experiment of Carbonate-Hydrogen Sulfide Equilibrium System and Its Geological Significance

ZHANG Shanming;QIN Shan;LIU Bo;WU Xiang;ZHANG Xuefeng;LIU Jianqiang;TIAN Yongjing;School of Earth and Space Sciences,Peking University;Center for High Pressure Science and Technology Advanced Research;Institute of Oil and Gas,Peking University;School of Earth Sciences and Resources,China University of Geosciences;  
The interactions between carbonate and H2 S saturated acid fluid at various temperatures and pressures in-situ conditions were simulated using hydrothermal diamond-anvil cell equipment combined with Raman spectroscopy. The heating process is from room temperature to 230℃ and then the system is cooled to room temperature again. Experimental results clearly demonstrate that carbonate minerals present much precipitation from room temperature to 140℃ and little precipitation from 140℃ to 230℃. Carbonate trends to precipitate with the increase of temperature and pressure, and dolomite is more stable than calcite and limestone. But in the cooling process carbonate suffers from little dissolution. So in the burial process, carbonate trends to precipitate, and the rapid closed burial and slow uplift process is beneficial to form high quality reservoirs in the deep closed condition. Fault and magmatic hydrothermal activities may break the closed system, which needs further study.
【Fund】: 国家科技重大专项(2011ZX05005-003-010HZ);; 国家自然科学基金(41272137)资助
【CateGory Index】: P618.13
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