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《Acta Sedimentologica Sinica》 2008-02
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Effect of Uranium Substance on Hydrocarbon Generation from Mudstone by Hydrous Pyrolysis

LU Hong-xuan1,2 MENG Zi-fang1 LI Bin1,2 LI Xiang-bo1,2 ZHENG Min1,2(1.Key Laboratory of Gas Geochemistry,Institute of Geology and Geophysics,Chinese Academy of Sciences,Lanzhou 730000;2.Graduate School of the Chinese Academy of Sciences,Beijing 100039)  
Organic-inorganic interactions are ubiquitous and unalterable in sedimentary basin.In this paper,effect of uranium substance on the mudstone pyrogenation was studied by hydrous pyrolysis.From the experiments,huge increase of the gas yields was observed.Further investigations showed that the content of carbon dioxide increased,while the content of methane decreased,and carbon monoxide was one of the metastable intermediates during the hydrous pyrolysis.At the same time,the high molecular weight hydrocarbons seemed to be more degraded by the uranium substance.The generated sterane and terpane from the hydrous pyrolysis were also affected by the uranium substance.
【Fund】: 国家重点基础研究发展规划项目(编号:40334038);; 中国科学院知识创新重要方向项目(编号:KZCX3-SW-147)资助
【CateGory Index】: P618.13
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