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《Geochimica》 2004-06
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Geochemical characteristics and or igin of Feixianguan Formation oolitic shoal natural gases in northeastern Sichuan basin

XIE Zeng-ye 1,2 ,TIAN Shi-cheng 1 ,LI Jian 2 ,HU Guo-yi 2 ,LI Zhi-sheng 2 ,MA Cheng-hua 2 1.School of Energy Resources,China University of Geosciences,Beijing100083,China;2.Langfang Branch,Research Institut e of Petroleum Exploration and Development,Langfang065007,China Correspondence should be addressed to XIE Zeng-ye(E-mail:xiezengye69@petrochina.com.cn)Received January 13,2004;revised April 17,2004;accepted May 8,2004;published November,2004  
Hydrocarbons in oolitic reservoir g ases of Feixianguan Formation in northeastern Sichuan basin mainly consist of methane with 75%-90%of CH 4 ,0%-0.15%ofC 2 + ,and the ratio of C 1 /(C 1 -C 5 )is 0.9970-0.9998.It is a typical dry gas.Nonhydrocarbon mainly consists of H 2 S and CO 2 ,and their relative contents are5%-20%and 1%-10%,respectively.The isotope composition of C 1 ranges from -29.0‰to -31.5‰,while that of C 2 from -29.4‰to -32.4‰.The oolitic re servoir gases are associated with th e sapropelic organic matter.The high sulfur-bearing gas distribution area is identical to th e gypseous distribution area.The H 2 S in natural gases is formed by thermochemical sulfate reduction(TSR),and the CO 2 is the main by-product of TSR.During TSR,the C 2 -C 5 hydrocarbon gases take priority of r eaction with sulfates over methane.Therefore,the natural gases that undergo TSR lack C 2 -C 5 hydrocarbons but contain methane,H 2 S,and other nonhydrocarbon gases,such as carbon dioxide.There is an inverse correlation betweenδ 13 C 1 and the absolute concentration of methane,which shows that a methane i s replaced by other gases(mainly H 2 S and CO 2 ),and the remaining methane becomes isotopically heavier.There is also a fairly well correlation between gas sourness犤H 2 S /(H 2 S +C n H 2n+2 )犦andδ 13 C 1 ,suggesting that TSR has directly ca used an alteration of the carbon isotope compositions of the remaining methane.The positive relationship between methaneδ 13 C 1 values and gas sourness leads to the i nference that as sulfate reduction of methane procee ded,12 C in methane was more rapidly deplete d than 13 C as a result of kinetic isotope fractionation with the residual methane becoming more enriched in 13 C.
【Fund】: “十五”国家重点科技攻关项目(2001BA605A-04);; 中国石油天然气集团公司天然气成藏与开发重点实验室资助项目
【CateGory Index】: P618.13
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