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《Geochimica》 2004-06
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Occurrence of REE at REE extra-enric hed bed in Pingba dolomite weathering crust,Guizhou Province,China

LI Yan-li 1,2 ,SUN Cheng-xing 3 ,WANG Shi-jie 1 ,LIU Xiu-ming 1 1.State Key Laboratory of Environment Geochemistry,Institute of Geochem istry,Chinese Academy of Sciences,Guiyang550002,China;2.Graduate School of Chinese Academy o f Sciences,Beijing100039,China;3.State Key Laboratory of Estuarine and Coastal Research,East China Norma l University,Shanghai 200062,China Correspondence should be addressed to WANG Shi-jie(E-mail:sjwang@ms.gyig.ac.cn)Received November 18,2003;revised March 6,2004;accepted April 8,2004;published November,2004  
Behavior and fractionation of REE at a REE extra-enriched bed near the soil-rock boundary in Pingba weathering profile have been studie d by chemical sequential extraction experiment and TEM observation.REE in the profile was partitioned into six fractions including soluble and exchangeable(Ⅰ),carbonate and adsorbed(Ⅱ),amorphous Fe-Mn oxide(Ⅲ),crystalline Fe-Mn oxide(Ⅳ),organics and sulfide(Ⅴ),and residual(Ⅵ).The statesⅡ,ⅤandⅥprevail at the REE extra-enriched bed.Acid-soluble REEs are dominant in the weathering frontier,making REEs easy to migrate downwards and transfer into other s tates(for example,StateⅡ)during weathering process.The secondary mineral of rare earth phosphates form ed by weathering of primary phosphor-containing mineral in dolomite was f ound to be accumulated in the weathering frontier and was the major compon ents in the stateⅥ.With the progressive weathering an d leaching,the soluble REE leached f rom the upper profile can co-precipitate with organics,Fe-M n oxides and clay minerals under the h igh pH values near soil-rock boundary,leading to the formation of the REE extra-enriched bed at Pingba,Guizhou Province.
【Fund】: 中国科学院地球化学研究所知识创新工程领域前沿项目(IG0401);; 国家自然科学基金(4027301540371012);; 中国科学院“西部之光”资助项目
【CateGory Index】: P618.7
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