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《Chinese Journal of Atmospheric Sciences》 2001-01
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A Study of Using Look-up Table Method to Simulate Tropospheric Ozone and NO_x Evolution and Their Distributions

Zhu Bin, Xiao Hui, Huang Meiyuan and Li Zihua (Nanjing Institute of Meteorology, Nanjing 2100044) (State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beiji  
Using STEM-II gas phase photochemistry model, the main physical/ chemical factors which influence the photochemical transformation of tropospheric O3 and NOx have been discussed. The results show that strength of solar radiation flux, temperature, the concentration of NOx and the concentration of initial O3 are important factors considering the features of photochemistry contamination in China. Then, the look-up tables of O3 and NOx are respectively constructed by calculating the rate of photochemical transformation of O3 and NOx in various conditions according to these factors. These tables are coupled with the dynamic frame of the STEM-II model to simulate the evolution and distribution of the tropospheric O3 and NOx over East Asia. The results by this method are in pretty good agreement with those directly by using the original STEM-II gas phase photochemistry model, and this model can highly save computation time and keep the basic features of strong non-linear processes in atmospheric chemical reactions.
【Fund】: 中国科学院“九五”重大项目!KZ951-A1-403-01
【CateGory Index】: P421.31
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