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《Environmental Science & Technology》 2010-01
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Oxidation of Active Red X-3B with Particles Electrodes Using Three Dimensional Electrolysis

LIU Zhan-meng1,HU Feng-ping1,LI Jing2,WANG Xiao-miao1(1.School of Civil Engineering and Architecture,East China Jiaotong University,Nanchang 330013,China;2.Department of Architecture Engineering,Xingtai Vocational and Technical College,Xingtai 054035,China)  
Particles electrodes of Cu/γ-Al2O3,Cu-Co/γ-Al2O3 were prepared by wet impregnation-roasting method.A novel three dimensional electrolysis system with TiO2/Ti as anodes and graphite as cathodes was introduced to treat Active Red X3B solution which was used as simulated dyestuff.Effects of particles electrodes,applied voltage,pH value and electrolyte concentration on removal efficiency of TOC and X-3B were investigated.Experimental results indicated that the electrocatalytic oxidation process could efficiently remove and degrade X-3B and the particles electrodes improved electrochemical oxidation efficiency.Compared with the particles electrodes of Cu/γ-Al2O3,Cu-Co/γ-Al2O3 showed a higher catalysis.The removal mechanism could be attributed to both indirect oxidation of hydroxyl radicals generated in electric catalysis system and direct oxidation on the interface of particles electrodes.
【Fund】: 江西省教育厅基金(GJJ08248);; 河北省建设科学技术研究计划项目资助(2008-142);; 华东交通大学校级课题(07TM08)
【CateGory Index】: X703
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