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《Environmental Science & Technology》 2010-12
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Catalytic Oxidation Degradation of Cationic Red GTL Simulated Wastewater by NiO-Al_2O_3

MA Feng1,HUANG Zi-li1,ZHANG Ya-ping2(1.School of Resource and Environment Engineering,Wuhan University of Science and Technology,Wuhan 430081,China;2.School of Biological Engineering,Jimei University,Xiamen 361021,China)  
NiO-Al2O3 catalysts were prepared via immersion method,as cationic red GTL simulated wastewater for subject,effects of ozone dosage,catalyst dosage,different processes on the cationic red GTL removal rate and CODCr were investigated,and stability of catalysts were investigated by experiment of recycling. Reaction mechanism of removal of cationic red GTL by catalytic oxidation were preliminary studied,which by the addition of inorganic anion,tertiary butanol and using of UV-Vis absorption spectrum. Results showed that removal rate of cationic red GTL of 100mg/L was 98.48%,CODCr removal rate was 78.79% after 14min reaction under the condition of ozone dosage 1.75g/h,NiO-Al2O3 catalysts dosage 0.5g/L,pH 7.0. In the catalysts recycling process,its activity could keep stable. The removal of dyes was retard by the addition of Cl-and SO42-while added CO32-could greatly accelerate the removal rate of the cationic red GTL. Hydroxyl radical played an important role on removal process of the cationic red GTL by O3/NiO-Al2O3 system.
【Fund】: 福建省科技计划项目(2008F5036);; 福建省青年创新人才项目(2008F3076);; 福建省自然科学基金项目(2009J01033);; 集美大学优秀骨干教师项目(2008C004)
【CateGory Index】: X703
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