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《Acta Photonica Sinica》 2011-04
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Third-order Nonlinear Optical Properties Study of [(C_3H_7)_4N][Au(C_3S_5)_2] Applied to All-optical Switches

LI Guo-chao~a,REN Quan~a,WANG Xin-qiang~b,YANG Hong-liang~a,CHEN Jing-wei~a,CAI Ning-ning~b(a.School of Information Science and Engineering;b.State Key Laboratory of Crystal Materials,Shandong University,Jinan 250100,China)  
A novel novel dmit2-salt: [(C3H7)4N][Au(C3S5)2] was synthesized.Its acetonitrile solution with concentration 1.0 ×10-3 mol/L was prepared.The thin film with [(C3H7)4N][Au(C3S5)2]-doped in PMMA was fabricated spin-coating on a quartz substrate.The third-order optical nonlinearities of sample solution and film were investigated by using the laser Z-scan technique with 20 ps pulses width at 1 064 nm.The experimental results show that the third-order nonlinear susceptibility χ(3) improves an approximate 3 orders of magnitude by the PrAu film over the solution.The nonlinear refraction coefficient n2 and the third-order nonlinear susceptibility χ(3) of the PrAu film were obtained to be 1.76×10-15 m2/W and 9.37×10-10 esu,respectively.The results suggest that PrAu will be a promising material for all-optical switching devices.
【Fund】: 国家自然科学基金(No.60778037 No.50772059);; 高等学校全国优秀博士学位论文专项资金(No.200539)资助
【CateGory Index】: O437
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