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《Research of Environmental Sciences》 2006-01
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Photoelectrocatalytic Degradation of Oilfield Wastewater with High Content of Chlorine

LI Gui-ying,AN Tai-cheng,CHEN Jia-xin,CHEN Fan-zhong,FU Jia-mo,SHENG Guo-ying,YE Heng-peng (State Key Laboratory of Organic Geochemistry,Guangdong Key Laboratory of Environmental Resources Utilization and Protection,Guangzhou Institute of Geochemistry,Chinese Academy of Sciences,Guangzhou 510640,China)  
The photoelectrocatalytic degradation of oilfield wastewater containing high content of chlorine was studied in TiO_2 aqueous suspensions.The effect of different degradation technologies,such as photocatalysis,electro_oxidation, photoelectrocatalysis and photoelectrocatalysis/H_2O_2,on the COD_(Cr) removal efficiency of oilfield wastewater was compared.The results showed that COD_(Cr) removal efficiency of photoelectrocatalysis was much higher than photocatalysis and electro-oxidation alone.It is also interesting to note that a certain amount of active chlorine was produced and had an obvious enhancement effect on both electro-oxidation and photoelectrocatalytic degradation of oilfield wastewater.The COD_(Cr) removal efficiency of photoelectrocatalysis/H_2O_2 was the highest,and much of organic pollutants were completely mineralized in a short period in that H_2O_2 can easily produce ·OH radical under UV irradiation.The effects of various operating conditions,such as initial concentration of wastewater,applied cell voltage and initial pH,were also investigated in detail.It was shown that the degradation efficiency of oilfield wastewater would be comparatively low when initial concentration of COD_(Cr) is too high or too low,and that the degradation efficiency increased with the increase of applied cell voltage or the decrease of initial pH of the wastewater.
【Fund】: 国家自然科学基金资助项目(40302013);; 广东省自然科学基金资助项目(04002146);; 瑞典国际科学基金资助项目(W/3635-1)
【CateGory Index】: X741
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