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《Chinese Journal of Rare Metals》 2008-01
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Effects of Preparation Methods of ZrO_2-Al_2O_3 Mixed Supports on Properties of Palladium Based Catalysts for HDS

Cheng Xinsun1,Luo Laitao1,Lu Xun1,Zhang Xueli2 (1.Department of Chemistry,Nanchang University,Nanchang 330031,China;2. Jiangxi Vocational & Technical College Of Information Application,Nanchang 330043,China)  
ZrO2-Al2O3 mixed supports were prepared by impregnation(I) and sol-gel(S) methods separately.Influences of preparation methods on properties of Pd based catalysts for thiophene hydrogenation desulfurization(HDS) were studied.Prepared samples were characterized by means of XRD,H2-TPD,H2-TPR and NH3-TPD.Comparing with Pd/ZrO2-Al2O3(I) catalyst,Pd/ZrO2-Al2O3(S) catalyst had a higher dispersion of palladium and stronger interaction between palladium and mixed supports and more acid sites,which presented an increasing driving-force toward the catalyzed conversion of thiophene.The methods prepared supporte affected the property of Pt based catalysts for HDS.
【Fund】: 高等学校博士学科点专项研究基金(20040403001);; 江西教育厅科研基金;; 南昌大学分析测试基金资助项目
【CateGory Index】: TE624.55
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